You can best fly Barcelona-Madrid (1h) for 65 Euros return, tax incl., try Vueling Airlines:
http://www.vueling.com/
Bus (8h) should cost 45 Euros return (www.alsa.es). Its exhausting though. Train (6h) 120 Euros return (www.renfe.es). Flying is the best option. Vueling works great.
What to visit:
-In BCN: www.barcelona-tourist-guide.com
To move around: Metro de Barcelona. Info and map download here: http://www.tmb.net/en_US/home.jsp
-Around BCN: Sitges, Cadaqués, Roses, Figueres...France?
To get there: Short Distance Train ('Renfe Cercanías')-http://www.renfe.es/cercanias/barcelona/
-More: (Catalonia Official Tourism Site): http://www.gencat.net/turistex_nou/home_ang.htm
-In MAD:http://www.webmadrid.com
Best way to move around MAD: Metro de Madrid by far. Download the updated map here: http://www.metromadrid.es/
Buy a 10 trip ticket 'Metrobus' (6,15 Euros). Valid for metro and bus. Can be shared by more than one person. Can also be used from Madrid-Barajas Airport (old terminals T1,T2,T3 ) to the city for 0,62 cents/ride, the cheapest transfer ever 😊. In case you arrive to brand new T4 there's a free bus to the older ones.
-Around MAD: Segovia, Toledo (use train 'Renfe Cercanías')-http://www.renfe.es/cercanias/madrid/
-More: http://www.descubremadrid.com/en/index.asp
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Other possibilities:
-Rent a car to move around Catalonia at your ease (air conditioned!!)
-Consider also visiting Pamplona for San Fermín Fiestas (July 7th - 16th) . But DO NOT run the bulls. 😊
-If flying with Ryanair remember they fly to GIRONA airport, not Barcelona. See 'Barcelona Tourist Guide'
-Most museums are free on Sundays. One of my favourite hidden little treasures in Madrid is the Sorolla Museum, an impressionist painter and his own XIX century house-studio. Also free on Sundays. http://museosorolla.mcu.es/index.html (only in spanish, sorry)
Sorry for the telegram-style. Have fun.
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